Quantum control of exciton wave functions in 2D semiconductors.

Excitons-bound electron-hole pairs-play a central role in light-matter interaction phenomena and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing challenge in solid-state optics has been to achieve precise and scalable control over excitonic motion. We present a technique using nanostructured gate electrodes to create tailored potential landscapes for excitons in 2D semiconductors, enabling in situ wave function shaping at the nanoscale. Our approach forms electrostatic traps for excitons in various geometries, such as quantum dots, rings, and arrays thereof. We show independent spectral tuning of spatially separated quantum dots, achieving degeneracy despite material disorder. Owing to the strong light-matter coupling of excitons in 2D semiconductors, we observe unambiguous signatures of confined exciton wave functions in optical reflection and photoluminescence measurements. This work unlocks possibilities for engineering exciton dynamics and interactions at the nanometer scale, with implications for optoelectronic devices, topological photonics, and quantum nonlinear optics.

Electrically tunable quantum confinement of neutral excitons.

Confining particles to distances below their de Broglie wavelength discretizes their motional state. This fundamental effect is observed in many physical systems, ranging from electrons confined in atoms or quantum dots1,2 to ultracold atoms trapped in optical tweezers3,4. In solid-state photonics, a long-standing goal has been to achieve fully tunable quantum confinement of optically active electron-hole pairs, known as excitons. To confine excitons, existing approaches mainly rely on material modulation5, which suffers from poor control over the energy and position of trapping potentials. This has severely impeded the engineering of large-scale quantum photonic systems. Here we demonstrate electrically controlled quantum confinement of neutral excitons in 2D semiconductors. By combining gate-defined in-plane electric fields with inherent interactions between excitons and free charges in a lateral p-i-n junction, we achieve exciton confinement below 10 nm. Quantization of excitonic motion manifests in the measured optical response as a ladder of discrete voltage-dependent states below the continuum. Furthermore, we observe that our confining potentials lead to a strong modification of the relative wave function of excitons. Our technique provides an experimental route towards creating scalable arrays of identical single-photon sources and has wide-ranging implications for realizing strongly correlated photonic phases6,7 and on-chip optical quantum information processors8,9.

Freeform Electronic and Photonic Landscapes in Hexagonal Boron Nitride.

Atomically smooth hexagonal boron nitride (hBN) flakes have revolutionized two-dimensional (2D) optoelectronics. They provide the key substrate, encapsulant, and gate dielectric for 2D electronics while offering hyperbolic dispersion and quantum emission for photonics. The shape, thickness, and profile of these hBN flakes affect device functionality. However, researchers are restricted to simple, flat flakes, limiting next-generation devices. If arbitrary structures were possible, enhanced control over the flow of photons, electrons, and excitons could be exploited. Here, we demonstrate freeform hBN landscapes by combining thermal scanning-probe lithography and reactive-ion etching to produce previously unattainable flake structures with surprising fidelity. We fabricate photonic microelements (phase plates, grating couplers, and lenses) and show their straightforward integration, constructing a high-quality optical microcavity. We then decrease the length scale to introduce Fourier surfaces for electrons, creating sophisticated Moiré patterns for strain and band-structure engineering. These capabilities generate opportunities for 2D polaritonics, twistronics, quantum materials, and deep-ultraviolet devices.

Quantum scale anomaly and spatial coherence in a 2D Fermi superfluid.

Quantum anomalies are violations of classical scaling symmetries caused by divergences that appear in the quantization of certain classical theories. Although they play a prominent role in the quantum field theoretical description of many-body systems, their influence on experimental observables is difficult to discern. In this study, we discovered a distinctive manifestation of a quantum anomaly in the momentum-space dynamics of a two-dimensional (2D) Fermi superfluid of ultracold atoms. The measured pair momentum distributions of the superfluid during a breathing mode cycle exhibit a scaling violation in the strongly interacting regime. We found that the power-law exponents that characterize long-range phase correlations in the system are modified by the quantum anomaly, emphasizing the influence of this effect on the critical properties of 2D superfluids.

High-temperature pairing in a strongly interacting two-dimensional Fermi gas.

The nature of the normal phase of strongly correlated fermionic systems is an outstanding question in quantum many-body physics. We used spatially resolved radio-frequency spectroscopy to measure pairing energy of fermions across a wide range of temperatures and interaction strengths in a two-dimensional gas of ultracold fermionic atoms. We observed many-body pairing at temperatures far above the critical temperature for superfluidity. In the strongly interacting regime, the pairing energy in the normal phase considerably exceeds the intrinsic two-body binding energy of the system and shows a clear dependence on local density. This implies that pairing in this regime is driven by many-body correlations, rather than two-body physics. Our findings show that pairing correlations in strongly interacting two-dimensional fermionic systems are remarkably robust against thermal fluctuations.